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Fuzzi, S. (author), Baltensperger, U. (author), Carslaw, K. (author), Decesari, S. (author), Denier van der Gon, H.A.C. (author), Facchini, M.C. (author), Fowler, D. (author), Koren, I. (author), Langford, B. (author), Lohmann, U. (author), Nemitz, E. (author), Pandis, S. (author), Riipinen, I. (author), Rudich, Y. (author), Schaap, M. (author), Slowik, J.G. (author), Spracklen, D.V. (author), Vignati, E. (author), Wild, M. (author), Williams, M. (author), Gilardoni, S. (author)The literature on atmospheric particulate maffer (PM), or atmospheric aerosol, has increased enormously over the last 2 decades and amounts now to some 1500—2000 papers per year in the refereed literature. This is in part due to the enormous advances in measurement technologies, which have allowed for an increasingly accurate understanding of...article 2015
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Baklanov, A. (author), Schlünzen, K. (author), Suppan, P. (author), Baldasano, J. (author), Brunner, D. (author), Aksoyoglu, S. (author), Carmichael, G. (author), Douros, J. (author), Flemming, J. (author), Forkel, R. (author), Galmarini, S. (author), Gauss, M. (author), Grell, G. (author), Hirtl, M. (author), Joffre, S. (author), Jorba, O. (author), Kaas, E. (author), Kaasik, M. (author), Kallos, G. (author), Kong, X. (author), Korsholm, U. (author), Kurganskiy, A. (author), Kushta, J. (author), Lohmann, U. (author), Mahura, A. (author), Manders-Groot, A. (author), Maurizi, A. (author), Moussiopoulos, N. (author), Rao, S.T. (author), Savage, N. (author), Seigneur, C. (author), Sokhi, R.S. (author), Solazzo, E. (author), Solomos, S. (author), Sørensen, B. (author), Tsegas, G. (author), Vignati, E. (author), Vogel, B. (author), Zhang, Y. (author)Online coupled mesoscale meteorology atmospheric chemistry models have undergone a rapid evolution in recent years. Although mainly developed by the air quality modelling community, these models are also of interest for numerical weather prediction and regional climate modelling as they can consider not only the effects of meteorology on air...article 2014
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Mann, G.W. (author), Carslaw, K.S. (author), Reddington, C.L. (author), Pringle, K.J. (author), Schulz, M. (author), Asmi, A. (author), Spracklen, D.V. (author), Ridley, D.A. (author), Woodhouse, M.T. (author), Lee, L.A. (author), Zhang, K. (author), Ghan, S.J. (author), Easter, R.C. (author), Liu, X. (author), Stier, P. (author), Lee, Y.H. (author), Adams, P.J. (author), Tost, H. (author), Lelieveld, J. (author), Bauer, S.E. (author), Tsigaridis, K. (author), van Noije, T.P.C. (author), Strunk, A. (author), Vignati, E. (author), Bellouin, N. (author), Dalvi, M. (author), Johnson, C.E. (author), Bergman, T. (author), Kokkola, H. (author), Von Salzen, K. (author), Yu, F. (author), Luo, G. (author), Petzold, A. (author), Heintzenberg, J. (author), Clarke, A. (author), Ogren, J.A. (author), Gras, J. (author), Baltensperger, U. (author), Kaminski, U. (author), Jennings, S.G. (author), O'Dowd, C.D. (author), Harrison, R.M. (author), Beddows, D.C.S. (author), Kulmala, M. (author), Viisanen, Y. (author), Ulevicius, V. (author), Mihalopoulos, N. (author), Zdimal, V. (author), Fiebig, M. (author), Hansson, H.C. (author), Swietlicki, E. (author), Henzing, J.S. (author)Many of the next generation of global climate models will include aerosol schemes which explicitly simulate the microphysical processes that determine the particle size distribution. These models enable aerosol optical properties and cloud condensation nuclei (CCN) concentrations to be determined by fundamental aerosol processes, which should...article 2014
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Mann, G.W. (author), Carslaw, K.S. (author), Reddington, C.L. (author), Pringle, K.J. (author), Schulz, M. (author), Asmi, A. (author), Spracklen, D.V. (author), Ridley, D.A. (author), Woodhouse, M.T. (author), Lee, L.A. (author), Zhang, K. (author), Ghan, S.J. (author), Easter, R.C. (author), Liu, X. (author), Stier, P. (author), Lee, Y.H. (author), Adams, P.J. (author), Tost, H. (author), Lelieveld, J. (author), Bauer, S.E., (author), Tsigaridis, K. (author), van Noije, T.P.C. (author), Strunk, A. (author), Vignati, E. (author), Bellouin, N. (author), Dalvi, M. (author), Johnson, C.E. (author), Bergman, T. (author), Kokkola, H. (author), von Salzen, K. (author), Yu, F. (author), Luo, G. (author), Petzold, A. (author), Heintzenberg, J. (author), Clarke, A. (author), Ogren, J.A. (author), Gras, J. (author), Baltensperger, U. (author), Kaminski, U. (author), Jennings, S.G. (author), O'Dowd, C.D. (author), Harrison, R.M. (author), Beddows, D.C.S. (author), Kulmala, M. (author), Viisanen, Y. (author), Ulevicius, V. (author), Mihalopoulos, N. (author), Zdimal, V. (author), Fiebig, M. (author), Hansson, H.C. (author), Swietlicki, E. (author), Henzing, J.S. (author)This study examines the global variation in particle size distribution simulated by twelve global aerosol microphysics models to quantify model diversity and to identify any common biases against observations. Evaluation against size distribution measurements from a new European network of aerosol supersites shows that the mean model agrees...article 2013
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South African EUCAARI measurements: Seasonal variation of trace gases and aerosol optical propertiesLaakso, L. (author), Vakkari, V. (author), Virkkula, A. (author), Laakso, H. (author), Backman, J. (author), Kulmala, M. (author), Beukes, J.P. (author), van Zyl, P.G. (author), Tiitta, P. (author), Josipovic, M. (author), Pienaar, J.J. (author), Chiloane, K. (author), Gilardoni, S. (author), Vignati, E. (author), Wiedensohler, A. (author), Tuch, T. (author), Birmili, W. (author), Piketh, S. (author), Collett, K. (author), Fourie, G.D. (author), Komppula, M. (author), Lihavainen, H. (author), de Leeuw, G. (author), Kerminen, V.-M. (author)In this paper we introduce new in situ observations of atmospheric aerosols, especially chemical composition, physical and optical properties, on the eastern brink of the heavily polluted Highveld area in South Africa. During the observation period between 11 February 2009 and 31 January 2011, the mean particle number concentration (size range...article 2012
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de Brugh, J.M.J.A. (author), Schaap, M. (author), Vignati, E. (author), Dentener, F. (author), Kahnert, M. (author), Sofiev, M. (author), Huijnen, V. (author), Krol, M.C. (author)This paper presents the aerosol budget over Europe in 2006 calculated with the global transport model TM5 coupled to the size-resolved aerosol module M7. Comparison with ground observations indicates that the model reproduces the observed concentrations quite well with an expected slight underestimation of PM10 due to missing emissions (e.g....article 2011
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Kulmala, M. (author), Asmi, A. (author), Lappalainen, H.K. (author), Baltensperger, U. (author), Brenguier, J.-L. (author), Facchini, M.C. (author), Hansson, H.-C. (author), Hov, Ø. (author), O'Dowd, C.D. (author), Pöschl, U. (author), Wiedensohler, A. (author), Boers, R. (author), Boucher, O. (author), de Leeuw, G. (author), Denier van der Gon, H.A.C. (author), Feichter, J. (author), Krejci, R. (author), Laj, P. (author), Lihavainen, H. (author), Lohmann, U. (author), McFiggans, G. (author), Mentel, T. (author), Pilinis, C. (author), Riipinen, I. (author), Schulz, M. (author), Stohl, A. (author), Swietlicki, E. (author), Vignati, E. (author), Alves, C. (author), Amann, M. (author), Ammann, M. (author), Arabas, S. (author), Artaxo, P. (author), Baars, H. (author), Beddows, D.C.S. (author), Bergström, R. (author), Beukes, J.P. (author), Bilde, M. (author), Burkhart, J.F. (author), Canonaco, F. (author), Clegg, S.L. (author), Coe, H. (author), Crumeyrolle, S. (author), D'Anna, B. (author), Decesari, S. (author), Gilardoni, S. (author), Fischer, M. (author), Fjaeraa, A.M. (author), Fountoukis, C. (author), George, C. (author), Gomes, L. (author), Halloran, P. (author), Hamburger, T. (author), Harrison, R.M. (author), Herrmann, H. (author), Hoffmann, T. (author), Hoose, C. (author), Hu, M. (author), Hyvärinen, A. (author), Hõrrak, U. (author), Iinuma, Y. (author), Iversen, T. (author), Josipovic, M. (author), Kanakidou, M. (author), Kiendler-Scharr, A. (author), Kirkevåg, A. (author), Kiss, G. (author), Klimont, Z. (author), Kolmonen, P. (author), Komppula, M. (author), Kristjánsson, J.-E. (author), Laakso, L. (author), Laaksonen, A. (author), Labonnote, L. (author), Lanz, V.A. (author), Lehtinen, K.E.J. (author), Rizzo, L.V. (author), Makkonen, R. (author), Manninen, H.E. (author), McMeeking, G. (author), Merikanto, J. (author), Minikin, A. (author), Mirme, S. (author), Morgan, W.T. (author), Nemitz, E. (author), O'Donnell, D. (author), Panwar, T.S. (author), Pawlowska, H. (author), Petzold, A. (author), Pienaar, J.J. (author), Pio, C. (author), Plass-Duelmer, C. (author), Prévôt, A.S.H. (author), Pryor, S. (author), Reddington, C.L. (author), Roberts, G. (author), Rosenfeld, D. (author), Schwarz, J. (author), Seland, O. (author), Sellegri, K. (author), Shen, X.J. (author), Shiraiwa, M. (author), Siebert, H. (author), Sierau, B. (author), Simpson, D. (author), Sun, J.Y. (author), Topping, D. (author), Tunved, P. (author), Vaattovaara, P. (author), Vakkari, V. (author), Veefkind, J.P. (author), Visschedijk, A. (author), Vuollekoski, H. (author), Vuolo, R. (author), Wehner, B. (author), Wildt, J. (author), Woodward, S. (author), Worsnop, D.R. (author), van Zadelhoff, G.J. (author), Zardini, A.A. (author), Zhang, K. (author), van Zyl, P.G. (author), Kerminen, V.-M. (author), Carslaw, K.S. (author), Pandis, S.N. (author)In this paper we describe and summarize the main achievements of the European Aerosol Cloud Climate and Air Quality Interactions project (EUCAARI). EUCAARI started on 1 January 2007 and ended on 31 December 2010 leaving a rich legacy including: (a) a comprehensive database with a year of observations of the physical, chemical and optical...article 2011
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Laakso, L. (author), Vakkari, V. (author), Laakso, H. (author), Virkkula, A. (author), Kulmala, M. (author), Beukes, J.P. (author), van Zyl, P.G. (author), Pienaar, J.J. (author), Chiloane, K. (author), Gilardoni, S. (author), Vignati, E. (author), Wiedensohler, A. (author), Tuch, T. (author), Birmili, W. (author), Piketh, S. (author), Collett, K. (author), Fourie, G.D. (author), Komppula, M. (author), Lihavainen, H. (author), de Leeuw, G. (author), Kerminen, V.-M. (author), TNO Bouw en Ondergrond (author)In this paper, new long-term measurements of chemical composition and physical properties of atmospheric aerosols carried out on the eastern brink of the heavily polluted Highveld area in South Africa are introduced. As expected, a high variability of aerosol properties was observed. Optical properties of aerosol particles were found to be...article 2010
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Vautard, R. (author), Schaap, M. (author), Bergström, R. (author), Bessagnet, B. (author), Brandt, J. (author), Builtjes, P.J.H. (author), Christensen, J.H. (author), Cuvelier, C. (author), Foltescu, V. (author), Graff, A. (author), Kerschbaumer, A. (author), Krol, M. (author), Roberts, P. (author), Rouïl, L. (author), Stern, R. (author), Tarrason, L. (author), Thunis, P. (author), Vignati, E. (author), Wind, P. (author), TNO Bouw en Ondergrond (author)Recently several regional air quality projects were carried out to support the negotiation under the Clean Air For Europe (CAFE) programme by predicting the impact of emission control policies with an ensemble of models. Within these projects, CITYDELTA and EURODELTA, the fate of air quality at the scale of European cities or that of the...article 2009
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van Loon, M. (author), Vautard, R. (author), Schaap, M. (author), Bergström, R. (author), Bessagnet, B. (author), Brandt, J. (author), Builtjes, P.J.H. (author), Christensen, J.H. (author), Cuvelier, C. (author), Graff, A. (author), Jonson, J.E. (author), Krol, M. (author), Langner, J. (author), Roberts, P. (author), Rouil, L. (author), Stern, R. (author), Tarrasón, L. (author), Thunis, P. (author), Vignati, E. (author), White, L. (author), Wind, P. (author), TNO Bouw en Ondergrond (author)Long-term ozone simulations from seven regional air quality models, the Unified EMEP model, LOTOS-EUROS, CHIMERE, RCG, MATCH, DEHM and TM5, are intercompared and compared to ozone measurements within the framework of the EuroDelta experiment, designed to assess air quality improvement at the European scale in response to emission reduction...article 2007
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TNO Bouw en Ondergrond (author), Vautard, R. (author), van Loon, M. (author), Schaap, M. (author), Bergström, R. (author), Bessagnet, B. (author), Brandt, J. (author), Builtjes, P.J.H. (author), Christensen, J.H. (author), Cuvelier, C. (author), Graff, A. (author), Jonson, J.E. (author), Krol, M. (author), Langner, J. (author), Roberts, P. (author), Rouil, L. (author), Stern, R. (author), Tarrasón, L. (author), Thunis, P. (author), Vignati, E. (author), White, L. (author), Wind, P. (author)We examine whether seven state-of-the-art European regional air quality models provide daily ensembles of predicted ozone maxima that encompass observations. Using tools borrowed from the evaluation of ensemble weather forecasting, we analyze statistics of simulated ensembles of ozone daily maxima over an entire summer season. Although the model...article 2006
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de Leeuw, G. (author), Skjoth, C.A. (author), Hertel, O. (author), Jickells, T. (author), Spokes, L. (author), Vignati, E. (author), Frohn, L. (author), Frydendal, J. (author), Schulz, M. (author), Tamm, S. (author), Sorensen, L.L. (author), Kunz, G.J. (author), TNO Fysisch en Elektronisch Laboratorium (author)The flux ofnitrogen species from the atmosphere into the ocean, with emphasis on coastal waters, was addressed during the ANICE project (Atmospheric Nitrogen Inputs into the Coastal Ecosystem). ANICE focused on quantifying the deposition ofatmospheric inputs ofinorganic nitrogen compounds (HNO3, NO3-, NH3 and NH4+) into the North Sea and the...article 2003
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de Leeuw, G. (author), Ambelas Skjøth, C. (author), Hertel, O. (author), Jickells, T. (author), Spokes, L. (author), Vignati, E. (author), Frohn, L. (author), Frydendall, J. (author), Schulz, M. (author), Tamm, S. (author), Sørensen, L.L. (author), Kunz, G.J. (author)The flux of nitrogen species from the atmosphere into the ocean, with emphasis on coastal waters, was addressed during the ANICE project (Atmospheric Nitrogen Inputs into the Coastal Ecosystem). ANICE focused on quantifying the deposition of atmospheric inputs of inorganic nitrogen compounds (HNO3, NO3-, NH3 and NH4+) into the North Sea and the...article 2003
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Ambelas Skjoth, C. (author), Hertel, O. (author), Vignati, E. (author), Pedersen, B. (author), Klein, L. (author), de Leeuw, G. (author), Spokes, L. (author), Jickells, T. (author), Schulz, M. (author), Sorensen, L. (author), Schluenzen, K.H. (author), Tamm, S. (author), TNO Fysisch en Elektronisch Laboratorium (author)The ANICE (Atmospheric Nitrogen Inputs into the Coastal Ecosystem) project addressed the atmospheric deposition of nitrogen to the North Sea, with emphasis on coastal effects. ANlCE focused on quantifying the deposition of inorganic nitrogen compounds to the North Sea and the governing processes. An overview of the results from modelling and...article 2003
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TNO Fysisch en Elektronisch Laboratorium (author), de Leeuw, G. (author), Moerman, M.M. (author), Cohen, L. (author), Brooks, B. (author), Smith, M. (author), Vignati, E. (author)Aerosols have a large effect on climate and weather. They modulate the surface irradiance in clear sky conditions, but also modify the radiative properties of clouds. To assess the consequences of reduced surface irradiation due to aerosols for weather forecasting and climate, data on aerosol radiative effects and their spatial and temporal...conference paper 2003
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Hertel, O. (author), Ambelas Skjøth, C. (author), Frohn, L.M. (author), Vignati, E. (author), Frydendall, J. (author), de Leeuw, G. (author), Schwarz, U. (author), Reis, S. (author), TNO Fysisch en Elektronisch Laboratorium (author)The atmospheric chemistry and deposition model has been applied for calculation of nitrogen and sulphur depositions to the entire North Sea area for the year 1999. The total atmospheric nitrogen and sulphur depositions to the North Sea area were determined to 709 kton (kt) N and 551 kt S, respectively. Since the North Sea area was calculated to...article 2002
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de Leeuw, G. (author), Frohn, L.M. (author), Geernaert, G. (author), Jensen, B. (author), Jickells, T. (author), Kunz, G. (author), Lund, S. (author), Moerman, M. (author), Pedersen, B. (author), von Salzen, K. (author), Schulz, M. (author), Skjoth, C.A. (author), Spokes, L. (author), Tamm, S. (author), Vignati, E. (author), Cohen, L. (author), Hertel, O. (author), Klein, L. (author), Mueller, F. (author), Schluenzen, K.H. (author), Sorensen, L.L. (author), TNO Fysisch en Elektronisch Laboratorium (author)The aim of the atmospheric nitrogen inputs into the coastal ecosystem (ANICE) project is to improve transport-chemistry models that estimate nitrogen deposition to the sea. To achieve this, experimental and modelling work is being conducted which aims to improve understanding of the processes involved in the chemical transformation, transport...article 2001
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de Leeuw, G. (author), Cohen, L.H. (author), Frohn, L.M. (author), Geernaert, G.L. (author), Hertel, O. (author), Jensen, B. (author), Jickells, T. (author), Klein, L. (author), Kunz, G.J. (author), Lund, S. (author), Moerman, M.M. (author), Muller, F. (author), Pedersen, B. (author), von Salzen, K. (author), Schlnzen, H. (author), Schulz, M. (author), Skjoth, C.A. (author), Sorensen, L.L. (author), Spokes, L. (author), Tamm, S. (author), Vignati, E. (author), TNO Fysisch en Elektronisch Laboratorium (author)Terrestrial inputs of nitrogen are often dominated by riverine transport, especially in the winter (Sanders et al., 1997). However, the atmospheric contribution to the total land based nitrogen input has been reported to be on the order of 30 % for the total North Sea area (North Sea Task Force, 1993). The atmospheric nitrogen load is directly...bookPart 2001
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TNO Fysisch en Elektronisch Laboratorium (author), Vignati, E. (author), de Leeuw, G. (author), Berkowicz, R. (author)The Coastal Aerosol Transport (CAT) model was developed to study the evolution of aerosol particle size distributions and composition in the coastal environment. The model simulates such processes as particle production at the sea surface, mixing of particles through the boundary layer by turbulent diffusion, gravitational settling, and dry...article 2001
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de Leeuw, G. (author), Neele, F.P. (author), Hill, M.K. (author), Smith, M.H. (author), Vignati, E. (author), TNO Fysisch en Elektronisch Laboratorium (author)quantitative source function for sea spray aerosol produced by waves breaking in the surf zone was determined from data collected with optical particle counters at both sides of the surf zone at two locations on the Californian coast. Three optical particle counters were used to measure profiles at the base of a pier; a fourth instrument was...article 2000
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